After Croatia, Brazil face Austria in their final pre-World Cup friendly before taking on Switzerland, Costa Rica and Serbia in Group C in Russian Federation. He smashed the ball into the net from around five meters (yards) with his right foot.
Neymar ran behind the goal, in front of Anfield's legendary Kop End, and punched the air in obvious delight as he was mobbed by team-mates.
Here are three things we noticed about Croatia from their match against Brazil.
Neymar and Roberto Firmino scored to help Brazil beat Croatia 2-0 at Anfield on Saturday, in what was an interesting game for both teams.
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Neymar, the world's most expensive player following his blockbuster move from Barcelona previous year, had been sidelined since the end of February when he fractured his foot playing for PSG in a league victory against Marseille.
Facing a race to be fit for Brazil's World Cup opener against Switzerland on June 17, Neymar will get a chance to use Sunday's clash at Anfield to show he is ready to lead the five-time world champions in Russian Federation.
Neymar was introduced at the start of the second half, replacing Fernandinho for his first appearances since sustaining an ankle injury in February.
Coutinho also tried to leave Liverpool for Barcelona last summer, but the Reds held on to him for a further six months.
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Neymar marked his return from injury with the first goal in Brazil's win over Croatia at Anfield.
"Neymar is only human, but he came back above my expectations too", Tite said.
The press successful negated much of Brazil's play in the first half with usually marauding left-back Marcelo stuck playing long balls at times to switch the play out to Willian.
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